To use your Harmony Touch to control your PlayStation 3, you'll need to first pair it with a Logitech Harmony Adapter for PS3 (see answer 360023412813). Then, add your PlayStation 3 as a device on your Harmony account. Here's how:
NOTE: If you already have a PlayStation3 device in your account, the codes might need to be updated. To update the codes, you'll need to delete the device and then re-add it (see answer 360023412813).
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Log in to your account on myharmony.com.
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Select your Harmony Touch from the Welcome screen.
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Click Devices.
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Click Add Device.
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Enter "Sony" as the Manufacturer and "PlayStation3" as the Model Number, and then click Add.
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Click Yes to confirm your device.
You're now ready to add your PlayStation 3 device to an activity. For more information on Harmony Activities, see answer 360023412813.